Autors: Manikandan R., C. Justin Raj., Simon E. Moulton., Todorov, T. S., Kook Hyun Yu., Kim B C.
Title: High energy density heteroatom (O, N and S) enriched activated carbon for rational design of symmetric supercapacitors
Keywords: Carbon-based symmetric supercapacitors

Abstract: Carbon-based symmetric supercapacitors (SCs) are known for their high power density and long cyclability, making them an ideal candidate for power sources in new-generation electronic devices. To boost their electrochemical performances, deriving activated carbon doped with heteroatoms such as N, O, and S are highly desirable for increasing the specific capacitance. In this regard, activated carbon (AC) self-doped with heteroatoms is directly derived from bio-waste (lima-bean shell) using different KOH activation processes. The heteroatom-enriched AC synthesized using a pretreated carbon-to-KOH ratio of 1:2 (ONS@AC-2) shows excellent surface morphology with a large surface area of 1508 m2 g−1. As an SC electrode material, the presence of heteroatoms (N and S) reduces the interfacial charge-transfer resistance and increases the ion-accessible surface area, which inherently provides additional pseudocapacitance. The ONS@AC-2 electrode attains a maximum specific capacitance (Csp) of 342 

References

    Issue

    Chemistry–A European Journal, vol. 27, issue 2, pp. 669-682, 2021, Germany, Wiley-VCH GmbH, Weinheim, ISBN ISSN:1521-3765

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    Вид: статия в списание, публикация в издание с импакт фактор, публикация в реферирано издание, индексирана в Scopus